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1.
Indoor radon measurements were carried out in a total of 420 dwellings and 17 schools in Hail region of Saudi Arabia, using NTDs based radon dosimeters. The duration of the measurements was one year, from April 2008 to April 2009. The indoor radon concentrations varied from 4 to 513 Bq/m3 with an overall average of 45 Bq/m3 for all surveyed dwellings. These passive measurements were confirmed by the active measurements. The anomalous concentrations above 200 Bq/m3 were observed in 13 dwellings, representing 3.1 % of the total surveyed dwellings. In Inbowan village alone, it was found that 7.6 % of the dwellings have indoor radon concentration above 200 Bq/m3. The highest average indoor radon concentration of 64 Bq/m3 was found in Inbowan village while the lowest average of 24 Bq/m3 was found in Majasah village. The city of Hail showed an average indoor radon concentration of 49 Bq/m3. The average indoor radon concentration in one area located at the edge of the Aja Mountain in Hail city was 111 Bq/m3. The elevated indoor radon concentrations in many dwellings in the Hail region, prompted us to measure outdoor ground radon in such locations using gas monitor. It was found that radon concentrations at a depth of 0.5 m varied significantly from place to place ranging from 1.2 to 177 kBq/m3. The outdoor radon concentrations are generally correlated with the indoor radon measurements. Radon exhalations from construction materials and soil samples from the Hail region were also measured. It was found that radon exhalations from soil samples are higher than that of construction materials by a factor of at least 3 and reaching up to 11. These results indicate that soil is the main source of indoor radon. Geological interpretations of the results are also given.  相似文献   

2.
Radon measurements in soil and groundwater (springs, thermal springs and handpumps) were made in a variety of lithological units including major thrusts between Mandi and Manali in Himachal Himalaya. Analysis of radon data in light of lithological controls and influence of deep-seated thrusts has been made to elucidate the causative factors for anomalous emanation of radon. The lithological types include banded gneisses, schists, quartzite, granite, phyllites, volcanics and mylonites. The low-grade metasedimentries of Shali and Dharamsala generally show low and narrow range of radon concentration in water (5.6–13.4 Bq/l) as well as in soil (1.8–3.2 kBq/m3) except for the samples related to thrusts. On the other hand, sheared and deformed rocks of Chail and Jutogh show moderate radon content (average 5.03 kBq/m3, range 2.9–11.1 kBq/m3) in soil. However, the groundwater radon concentration shows wide variation in different types of sources (2.1–80.8 Bq/l). The quartzite and volcanic rocks of Rampur formation in this area present as a window separated by Chail thrust. Radon emanations on these rock types are relatively high (6.3–68.1 Bq/l in water and 5.5–15.9 kBq/m3 in soil) and are exceptionally high in samples that are related to uranium mineralization, deep-seated thrusts and hot springs (13.5–653.5 Bq/l). It is generally observed that anomalous high radon content is associated with mineralization, deeper source and tectonic discontinuities. Whereas it is obvious that subsurface radioactive mineralization would facilitate enhanced radon production, however, thrust plains provide easy pathways for escape of gases from the deeper sources. Shallow and deep sources of the groundwater have contrasting radon content particularly in the deformed and metamorphosed rocks of Jutogh and Chail. Shallow groundwater sources, mainly handpumps, have lower radon concentration due to limited superficial water circulation, whereas deeper sources, mainly perennial springs, show higher radon content because of larger opportunity for water–rock interaction.  相似文献   

3.
Radon measurements were made in the soil and spring/seepage water in and around an active landslide located along the Pindar river in the Chamoli District of Uttaranchal in Garhwal Lesser Himalaya, to understand the application of radon in geological disasters. The landslide is a compound slide i.e. a slump in the crown portion, and debris slide and fall in the lower part. The bedrock consists of gneisses and schists of the Saryu Formation of the Almora Group of Precambrian age. The presence of several small slump scars and debris slide/fall scars along the length of the slide indicates continuous downward movement. The radon concentrations in the present study are much lower in comparison to values reported from other regions. However, the present radon data show relative variation in the slide zone. The concentration of radon measured in landslide zones varies from 3.1 Bq/l to 18.4 Bq/l in spring water and from 2.3 kBq/m3 to 12.2 kBq/m3 in the soil gas of the debris. Along the section of the slide, the radon values in water and soil are slightly higher in the upper slopes i.e. toward the crown portion of the landslide as compared to the distal portion. The relatively low concentration of radon both in soil gas and water in the toe portion of the landslide may be due to the high porosity of the debris, which does not allow radon to accumulate in the soil and water, whereas, towards the crown portion, the high frequency of fractures increases the surface area due to particle size reduction, and the near absence of debris enhances the radon emanation in soil.  相似文献   

4.
Radon concentration was evaluated in dwellings of the urban area of Vila Real (Northern Portugal). The area is mainly composed of Hercynian granites and Cambrian metasediments, and CR-39 passive detectors (n = 112) were used for the purpose. The results obtained in winter conditions suggest that the most productive geological unit is the Hercynian granite G1 (geometric mean of 364 Bq/m3), while Cambrian metasediments of the Douro Group show the lowest average indoor radon concentration (236 Bq/m3). The geological, geochemical and radiological data obtained suggest that the most effective control on the radon concentrations of the area is related with the uranium content of the rocks; indeed, the highest contents were observed in granite G1 (21 ppm) and the lowest in the metasediments (3 ppm). This is also confirmed by the results obtained for groundwater, where granites present the highest concentrations of dissolved radon (up to 938 Bq/l), uranium (5–18 ppb) and gross α activities (0.47–0.92 Bq/l). No important radiometric anomalies were found in relation with geological structures such as faults, veins and contacts, but a moderate increase of the uranium content can occur locally in such structures. Petrographic observations and SEM studies show that uranium is mainly contained within the rock in heavy accessory minerals (apatite, zircon, monazite, xenotime), which reduces radon emanation. Notwithstanding, due to the high U contents granites show a significant potential to induce indoor radon concentrations in dwellings in excess of the recommended value of 400 Bq/m3. Overall, we can conclude that the region of Vila Real presents a moderate to high radon risk in dwellings and groundwater.  相似文献   

5.
周云龙  岑况  施泽明 《现代地质》2013,27(4):993-998
采用IED-3000R轻便型测氡仪,对四川阿坝地区土壤、空气中的氡气浓度开展初步调查。结果表明:(1)测区空气中氡气浓度较高,均在平均值185 Bq/m3附近;(2)所测得土壤的氡气浓度范围为2 736~93 486 Bq/m3,平均值为26 021 Bq/m3,远远高于全国城市土壤中氡气浓度7 300 Bq/m3的平均值,同时在156个土壤氡气浓度被测点中共有91个测点氡气浓度值超过20 000 Bq/m3,而按照国家标准,对于民用建筑工程土壤中氡气浓度超过20 000 Bq/m3要进行不同程度的防氡工程;(3)地质环境、土壤松散度、岩土性质、土壤含水率为影响阿坝地区土壤氡气浓度的主要因素。  相似文献   

6.
This study was conducted primarily to measure and map radon activity concentration in soil gas and to understand the effect of geology and lithology and meteorology on radon concentration. Portable radon meter has been used for the measurement of soil gas radon at 30 different locations around Uro and Korn area in eastern Nuba Mountain South Kordofan State. The results indicate that the activity concentrations of 222Rn in soil gas fall within the range of 20–1,359 Bq/m3 with geometric mean of 102.80 Bq/cm3. The obtained data show that samples around Uro have anomaly of 222Rn concentrations than the sample around Korn. The reason could be attributed to differences in the geological structure, lithology and climate parameters. GIS predicative map has shown that the elevated levels of radon concentration were measured in North study area. Upon comparing the results with global data, it was found that the obtained values are far below the reported range of India, Slovenia, Portugal and Syria. However, the range of 222Rn concentrations in the soil observed in this study is significantly high relative to similar data reported from Libya. The regression analysis has shown that no correlation was noted between radon concentrations, climatic parameters and trace element.  相似文献   

7.
This paper presents the results of radon concentration measurements in the drinking water from the municipal water supply system and private wells of Xian, Xianyang and Baoji city of Shaanxi province of China. The measurements were carried out on 38 samples. Radon levels in drinking water in Xian, Xianyang and Baoji were found to be 5.78, 13.04 and 15.01 k Bq m–3, respectively. The AM radon concentration of private well water from Xianyang and Baoji is 28.84 k Bq m–3 and 38.85 k Bq m–3, respectively, which is 2.56 times and 3.14 times as high as that of tap water radon, respectively. The radiation risk of radon in water would be due to degassing and not due to drinking water. The domestic use of showers, humidifiers, and cooking, washing up, laundering, etc. may lead to an additional increase of the radon concentration in the indoor air. The observed radon concentration in drinking water from three main cities of Shaanxi Province can contribute to a 4.86 to 32.63% increase in indoor radon concentration and can cause 0.068±0.016 mSv y–1 to 0.177±0.045 mSv y–1 extra annual effective dose to males, 0.060±0.014 mSv y–1 to 0.155±0.039 mSv y–1 to females. The mean annual effective dose equivalents to males and females of Xianyang and Baoji from well water account for 25.94 to 39.75% of environmental radon and radon daughters annual effective dose equivalents. The radon concentrations in the well water from Xianyang and Baoji will bring a definite additional risk to the population.  相似文献   

8.
In 1996–1997, indoor radon values of more than 40,000 Bq/m3 and large seasonal and geographical variations in indoor air radon were reported from a residential area located on a highly permeable ice-marginal deposit. Geochemical analyses of bedrock, groundwater and sediments and comparisons between indoor radon values and soil radon values indicate that the indoor radon concentrations in this area are strongly affected by subterranean airflows caused by temperature differences between soil air and atmospheric air. The airflows concentrate the radon-laden soil air towards the topographic highest part of the deposit in winter and towards the topographic lowest part in summer. In areas where subterranean airflows are likely to occur, radon measurements performed both in summer and in winter provide the best estimate of annual average indoor radon concentrations, and assessments of indoor radon concentrations based on single soil gas measurements are not recommended.  相似文献   

9.
Radon is a radioactive hazardous and ubiquitous gas. It has been recognized to be one of the major contributors to natural radiation even causing lung cancer if present at enhanced levels. There are large variations in data available in the literature for radium content and radon exhalation rates of various materials. It is a well-documented fact that radon exhalation from the ground surface depends upon a number of parameters such as soil grain size, soil porosity and radium content. For this purpose, in this study the so-called can technique has been used to measure radium content and exhalation rates of radon in soil samples collected from different places of Aligarh, Etah and Mathura districts of Uttar Pradesh??a province in northern India. These districts lie within the subtropical region of the Indo-Gangetic plains. The values of effective radium content are found to vary from 8.11 to 112.83?Bq?kg?1 with a mean value of 33.21?Bq?kg?1 and a standard deviation of 28.15. The values of mass exhalation rates of radon vary from 0.76?×?10?6 to 15.80?×?10?6?Bq?kg?1?day?1 with a mean value of 4.21?×?10?6?Bq?kg?1?day?1, while the surface exhalation rates vary from 1.97?×?10?5 to 41.03?×?10?5?Bq?m?2?day?1 with a mean value of 10.93?×?10?5?Bq?m?2?day?1.  相似文献   

10.
Soil radon (222Rn) has been monitored during winter months under cool-temperate deciduous stands of different surface geology in Tomakomai and in Sapporo, Hokkaido, Japan. Radon level was lower in Tomakomai of immature soil of porous volcanic ash emitted from an active volcano (Mt. Tarumae), compared with those in Sapporo of alluvial sediments. In Tomakomai, mean value of the 222Rn activity concentration was higher in winter (570 Bq m?3) than in summer (350 Bq m?3) at a depth of 1 m, which is consistent with the results in cold and dry winter reported in the literature. In contrast, soil radon decreasing with decreasing soil temperature from mid-September (5.0 kBq m?3) remained low (2.6 kBq m?3) under persistent snow in Sapporo, which had already been observed in the same location. Measurements of the activity concentrations of 222Rn in snow and in snow air as well as in soil air indicate that the small amount of 222Rn is released from the ground surface to the overlying snowpack with a 222Rn flux density of 0.4 mBq m?2 s?1 under thick snow cover in Sapporo.  相似文献   

11.
The region of Amarante (Northern Portugal) is composed of Hercynian tardi-tectonics granites and Paleozoic metasediments. Petrographic observations and SEM studies show that uranium is mainly contained within the rock in heavy accessory minerals such as apatite, zircon, monazite, uraninite, thorite and thorianite. The geological, geochemical and radiological data obtained suggest that the radon concentrations in dwellings of the studied area are mainly related with the uranium content of the rocks. Indeed, the highest contents were observed in granite AT2 of Padronelo (18.2 ppm) and the granite AT1 of Telões (10.3 ppm), with metasediments showing much lower uranium contents of 1.6 ppm; radon concentrations were evaluated in dwellings, using CR-39 passive detectors, and the results obtained in winter conditions suggest that the most productive geological units are the granites AT2 and AT1, with geometric means of 430 and 220 Bq/m3, respectively, while the metasediments show the lowest value of 85 Bq/m3. Some moderate radiometric anomalies, where uranium contents can double typical background values, were found in relation with specific fault systems of the region affecting granitic rocks, thus increasing radon risk; this is an indication of uranium mobility, likely resulting from the leaching of primary mineral supports as uraninite. Groundwater radionuclide contents show a wide range of results, with the highest activities related with granitic lithologies: 2,295 Bq/l for radon, 0.83 Bq/l for gross α and 0.71 Bq/l for gross β, presenting metasediments much lower values, in good agreement with other results obtained. Absorbed dose measured with gamma spectrometers in direct contact with the rocks is directly related with the uranium contents of the rocks, and thus works as a fast proxy for radon risk. It is concluded that radon risk is moderate to high in the granitic areas of the Amarante region and low in the metasediments of the same region.  相似文献   

12.
 Generalized geologic province information and data on house construction were used to predict indoor radon concentrations in New Hampshire (NH). A mixed-effects regression model was used to predict the geometric mean (GM) short-term radon concentrations in 259 NH towns. Bayesian methods were used to avoid over-fitting and to minimize the effects of small sample variation within towns. Data from a random survey of short-term radon measurements, individual residence building characteristics, along with geologic unit information, and average surface radium concentration by town, were variables used in the model. Predicted town GM short-term indoor radon concentrations for detached houses with usable basements range from 34 Bq/m3 (1 pCi/l) to 558 Bq/m3 (15 pCi/l), with uncertainties of about 30%. A geologic province consisting of glacial deposits and marine sediments was associated with significantly elevated radon levels, after adjustment for radium concentration and building type. Validation and interpretation of results are discussed. Received: 20 October 1997 · Accepted: 18 May 1998  相似文献   

13.
In the Alban Hills area, strong areally diffuse and localised spot degassing processes occur (Tivoli, Cava dei Selci, Solforata, Tor Caldara). The gas comprises a large proportion of CO2, with minor CH4, H2S and Rn. These advective features are generated by fluid leakage from buried reservoirs hosted in the structural highs of the Mesozoic carbonate basement. Gas migration towards the surface is controlled by fault and fracture systems bordering the structural highs of the carbonate formations (e.g. Ciampino high). His release is triggered when the total pressure of the fluid phase exceeds the hydrostatic pressure, thus forming a free gas phase. Furthermore, both the sudden and catastrophic, and slow and continuous gas release at surface, of naturally occurring toxic species (CO2, H2S and Rn) poses a serious health risk to people living in this geologically active area.This paper presents data obtained from soil gas and gas flux surveys, as well as gas isotopes analyses, which suggest the presence of a deep origin gas flux enriched in carbon dioxide and minor species (CH4 and H2S), as well as a channelled migration of geogas mixtures having a Rn component which is not produced in situ.In regards to the health risk to local inhabitants, it was found that some anomalous areas had been zoned as parkland while others had been heavily developed for residential purposes. For example, many new houses were found to have been built on ground which has soil gas CO2 concentrations of over 70% and a CO2 flux of about 0.7 kg m−2 day−1, as well as radon values of more than 250 kBq/m3. In addition, an indoor radon survey has been conducted in selected houses in the town of Cava dei Selci to search for a possible correlation between the local geology and the radon concentration in indoor air. Preliminary results indicate high indoor values at ground floor levels (up to 1000 Bq/m3) and very high values in the cellars (up to 250.000 Bq/m3). It is recommended that land-use planners incorporate soil gas and/or gas flux measurements in the environmental assessment of areas of possible risk (i.e. volcanic or structurally active areas).  相似文献   

14.
Soil gas radon measurements were made in Chamba and Dharamshala regions of Himachal Pradesh, India, to study the correlation, if any, between the soil gas radon, radium activity concentration of soil, and the geology/active tectonics of the study region. Soil gas radon surveys were conducted around the local fault zones to check their tectonic activities using the soil gas technique. Soil gas radon activity concentration at thirty-five different locations in Dharamshala region has been found to be varying from 13.2 ± 1.5 to 110.8 ± 5.0 kBq m?3 with a geometrical mean of 35.9 kBq m?3 and geometrical standard deviation of 1.8. Radon activity concentration observed in the thirty-seven soil gas samples collected from the Chamba region of Himachal Pradesh varies from 5.2 ± 1.0 to 35.6 ± 2.5 kBq m?3, with geometrical mean of 15.8 kBq m?3 and geometrical standard deviation of 1.6. Average radium activity concentrations in thirty-four soil samples collected from different geological formations of Dharamshala region and Chamba region are found to be 40.4 ± 17 and 38.6 ± 1.7 Bq kg?1, respectively. It has been observed that soil gas radon activity concentration has a wide range of variation in both Dharamshala and Chamba regions, while radium activity concentrations in soil samples are more or less same in both the regions. Moreover, soil gas radon activity concentration has a better positive correlation with the radium activity concentration in soil samples collected from Chamba region as compared to Dharamshala region.  相似文献   

15.
This work presents the results of a soil erosion study using the 7Be technique. This technique estimates the water erosion/deposition from the comparison between 7Be soil content of a reference site and an eroded or sedimented site. The soil samples were collected from an agricultural area of the semiarid region of Argentina near San Luis City, which has a marked rainfall season. The area has been used for crop cultivation, being subjected to plowing practices. The 7Be in the Reference Site was in the first centimeter of soil, showing the typical exponential decreasing of 7Be soil content with depth, with the 7Be inventories value being 340?±?50 Bq m?2 for the dry season and 571?±?48 Bq m?2 for the rainy season. The 7Be technique was applied to a potential eroded site subjected to traditional tillage practices (plowing). A net soil erosion value of 13.5 t ha?1 (1.35 kg m?2) was obtained. From the assumptions of the applied technique, we can draw the inference that this erosion was caused by rains produced in the month prior to the date of soil sampling.  相似文献   

16.
The study was conducted for the investigation of amount of radioactivity in the barren and cultivated soil of Bio saline Research Station in Pakka Anna, established by Nuclear Institute for Agriculture and Biology (NIAB) in 1990, 34 km. away from the city of Faisalabad, in the Punjab province of Pakistan. The studies were done on an area of about 100 hectares of two types of virgin and fertilized saline soils. The technique of gamma ray spectrometry was applied using HPGe (high purity germanium) gamma ray detector and a PC based MCA. Activity concentration levels due to 40K, 137Cs, 226Ra and 232Th were measured in 250 saline soil samples collected at a spacing of about 4 hectares at the depth level of 0–25 cm. with a step of 5 cm. depth. Activity concentrations ranges of the concerned radionuclides for both of the soils were as follows: 40K, for virgin and cultivated saline soil was 500–610.2 and Bq/kg 560.2–635.6 respectively; 137Cs, 3.57–3.63 and 1.98–5.15 Bq/kg 238U, 26.3–31.6 and 30.3–38.7 Bq/kg, and 232Th, 50.6–55.3 and 50.6–64.0 Bq/kg respectively. The absorbed dose rate in air lies in the region 63–73 nGyh-1 and 68–83 nGyh-1 for virgin and fertilized soils respectively. This indicates that this region lies in the area of higher radiation background, while comparing with the worlds’ average. The slightly higher value of dose in the fertilized farm may be due to the use of fertilizers for cultivation. Before the radiometric measurements, chemical analysis for concentration of Na, Ca and Mg was also carried out along with the measurement of electrical conductivity and pH of the soil samples.  相似文献   

17.
Soil-gas radon measurements provide a valuable tool in assessing probable indoor radon levels on a regional basis. However, in Great Britain, seasonal weather changes can cause large changes in soil-gas radon concentration. Although this does not significantly constrain systematic radon potential mapping programmes, it does cause difficulties in responding to ad-hoc requests for site-specific radon investigations. The relationship between soil-gas radon and gamma spectrometry measurements made in the field with radon released from a representative sample of soil in the laboratory has been investigated as part of a program to develop a method of radon potential mapping and site investigation which can be used at any time of the year. Multiple soil and soil-gas samples were collected from sites underlain by bedrocks with widely varying radon potentials. For each geological unit, sites both free of and covered by glacial drift deposits were sampled. Soil and soil-gas samples were taken at the same depth of 60–100 cm. The effectiveness of these radon site investigation procedures has been evaluated by studying the relationship between the soil-gas radon, gamma spectrometry and radon emanation data with an independent estimate of the radon risk. The geologic radon potential (GEORP), which is the proportion of existing dwellings which exceed the UK radon Action Level (200 Bq m−3) for a particular combination of solid and drift geology within a defined geographic area, has been used for this study as the independent estimate of radon risk. Soil-gas radon, radon emanation and eU (equivalent uranium by field γ spectrometry) are all good geochemical indicators of radon risk (GEORP) in Derbyshire but only soil-gas radon correlates significantly with GEORP in Northamptonshire. Radon in soil gas discriminates more effectively between sites with different radon potential in Northamptonshire if soil permeability is also taken into account. In general, measurement of soil-gas radon in the field provides the most universally applicable indicator of radon potential. If soil-gas radon concentrations cannot be determined because of climatic factors, for example when the soil profile is waterlogged, measurement of radon emanation in the laboratory or measurement of eU can be used as radon potential indicators in some geological environments. This applies particularly in areas where the soil composition rather than the composition and permeability of the underlying rock or superficial deposits are the dominant controls of radon potential. It appears, therefore, that it may be necessary to use different radon site investigation methods according to the specific factors controlling radon emanation from the ground. In some cases no method will provide a reliable indicator of radon risk under unfavourable climatic conditions.  相似文献   

18.
Radon gas is a human health hazard; long-term exposure to high radon concentrations through inhalation is the second leading cause of lung cancer. Nova Scotia has been previously identified as a potential high risk region because of the geology. As such, the gas transport through Halifax’s fine grained leucomonzogranite (FGL) unit of the South Mountain Batholith needed to be quantified to further remediation efforts. Using controlled laboratory experiments, four different soil columns were created using the Halifax Regional Municipality’s (HRM) highest producing field tills and bedrock. Permeability, diffusivity, radon-222 gas concentrations, and gas transit time/speed were measured in both dry tills (field moisture) and wet tills (simulated rain event moisture). Columns with HRM till displayed the highest radon concentrations, and were less permeable with additional moisture. Radon diffusivity calculated from CO2 was 7.52 × 10?8 m2 (dry), and 3.37 × 10?8 m2 (wet); diffusivity calculated from 222Rn was 7.30 × 10?7 m2 (dry), and 6.47 × 10?7 m2 (wet). The average FGL transit time in a 60 cm column was 3.57 days (dry), and 3.82 days (wet). Locally this study presents two different methods for diffusivity calculations, for a unit lacking previous diffusivity information. The radon gas concentrations and transport speeds quantified the transport mechanisms within the till. Globally, the correlation between soil moisture, and radon/permeability values was established using these results. The link between diffusivity and permeability was also confirmed using field tills. Implications were made for building foundations, as well as the depth and type of material necessary to reduce radon gas from reaching the surface.  相似文献   

19.
 Radon concentration was measured in 133 water samples from tubewells, handpumps, dug wells and springs of the Doon Valley, Outer Himalaya, India. The observed radon values were found to vary from 10 to 154 Bq/l whereas radium in selected water samples varied from 0.11 to 0.75 Bq/l. Three different clusters of high radon values were observed in the north-western, central and south-eastern parts of the Doon Valley. These clusters were found to be associated with tectonics (thrust/fault) and associated uranium mineralization in the area. In general, radon concentration in groundwater was found to be positively correlated with the depth of the wells, whereas no significant correlation was observed between radon concentration in groundwater and the water temperature, pH value, conductivity and altitude of the water samples. An attempt has also been made to determine the nature and extent of aquifers in the Doon Valley on radon concentration in groundwater. The variation in radon concentration within the groundwater of the study area was found to be controlled by the neotectonic activity and geohydrological processes that occur in the area. The impact of these activities on radon concentration in groundwater are discussed. Received: 17 September 1999 · Accepted: 11 April 2000  相似文献   

20.
Depth-discrete tracing of residual dense non-aqueous phase liquid (DNAPL) sources in the subsurface is of great importance in making decisions related to contaminated groundwater remediation. Temporal variations in the natural tracer 222Rn and contaminant concentrations in groundwater contaminated with multiple chlorinated contaminants, such as trichloroethene, carbon tetrachloride, and chloroform, were examined to trace residual multiple DNAPL contaminants at an industrial complex in Wonju, Korea. The 222Rn activities and multiple DNAPL concentrations in the groundwater fluctuated irregularly according to the groundwater recharge. The natural tracer 222Rn in groundwater present in the soil layer, originating from the underlying crystalline biotite granite, had a wide range from 29,000 to 179,000 Bq/m3, and total concentrations of chlorinated solvents ranged from 0.06 to 17.77 mg/l, indicating the ambiguous results of 222Rn for tracing the residual DNAPL sources. In this paper, a method is presented to locate zones with a high probability of containing depth-discrete residual multiple DNAPL sources using 222Rn and considering relative contaminant concentrations. The results demonstrate that the combination of the 222Rn activities as a natural tracer and the relative contaminant concentrations is able to be used as a useful tool for tracing residual DNAPLs.  相似文献   

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